FN Archimer Export Format PT J TI Distributions of total and size-fractionated particulate 210Po and 210Pb activities along the North Atlantic GEOTRACES GA01 transect: GEOVIDE cruise BT AF Tang, Yi Castrillejo, Maxi Roca-Martí, Montserrat Masqué, Pere Lemaitre, Nolwenn Stewart, Gillian AS 1:1,2;2:3,4;3:3;4:3,5;5:6;6:1,2; FF 1:;2:;3:;4:;5:;6:; C1 Earth and Environmental Sciences, the Graduate Center, City University of New York, New York, USA School of Earth and Environmental Sciences, Queens College, City University of New York, Flushing, USA Institut de Ciència i Tecnologia Ambientals & Departament de Física, Universitat Autònoma de Barcelona, Bellaterra, 08193, Spain Laboratory of Ion Beam Physics, ETH Zurich, Otto-Stern-Weg 5, Zürich, 8093, Switzerland School of Science and Centre for Marine Ecosystems Research, Edith Cowan University, Joondalup, Western Australia, Australia Department of Earth Sciences, Institute of Geochemistry and Petrology, ETH Zurich, Zürich, Switzerland C2 CITY UNIV NEW YORK, USA CITY UNIV NEW YORK, USA UNIV AUTONOMA BARCELONA, SPAIN ETH ZURICH, SWITZERLAND UNIV EDITH COWAN, AUSTRALIA ETH ZURICH, SWITZERLAND IF 3.951 TC 11 UR https://archimer.ifremer.fr/doc/00485/59671/62736.pdf https://archimer.ifremer.fr/doc/00485/59671/62737.pdf https://archimer.ifremer.fr/doc/00485/59671/62739.xlsx https://archimer.ifremer.fr/doc/00485/59671/62740.pdf https://archimer.ifremer.fr/doc/00485/59671/62741.pdf LA English DT Article CR GEOVIDE BO Pourquoi pas ? AB Vertical distributions of total and particulate polonium-210 (210Po) and lead-210 (210Pb) activities in the water column were measured at 11 stations in the North Atlantic during the GEOTRACES GA01 transect: GEOVIDE cruise in May–June 2014. Total 210Po activity was on average 24 % lower than 210Pb activity in the upper 100 m, and it was closer to unity in the mesopelagic (100–1000 m). The partitioning coefficients (Kd) along the transect suggest the preferential association of 210Po relative to 210Pb onto particles. The prominent role of small particles in sorption was confirmed by the observation that over 80 % of the particulate radionuclide activity was on small particles. To account for the observed surface water 210Po ∕ 210Pb disequilibria, particulate radionuclide activities and export of both small (1–53 µm) and large (>53 µm) particles must be considered. A comparison between the GEOVIDE total particulate 210Po ∕ 210Pb activity ratios (ARs) and the ratios in previous studies revealed a distinct geographic distribution, with lower particulate ARs in the high-latitude North Atlantic (including this study) and Arctic in relation to all other samples. For the samples where apparent oxygen utilization (AOU) was calculated at the same depth and time as the 210Po ∕ 210Pb AR (40 stations including this study), there was a two-phase correlation between the total particulate AR and AOU, likely reflecting the nature of the particles and demonstrating the forces of remineralization and radionuclide decay from particles as they age. PY 2018 PD SEP SO Biogeosciences SN 1726-4170 PU Copernicus GmbH VL 15 IS 17 UT 000444619000001 BP 5437 EP 5453 DI 10.5194/bg-15-5437-2018 ID 59671 ER EF